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Titlebook: Coherent Light-Matter Interactions in Monolayer Transition-Metal Dichalcogenides; Edbert Jarvis Sie Book 2018 Springer International Publi

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書目名稱Coherent Light-Matter Interactions in Monolayer Transition-Metal Dichalcogenides
編輯Edbert Jarvis Sie
視頻videohttp://file.papertrans.cn/230/229208/229208.mp4
概述Nominated as an outstanding Ph.D. thesis by Massachusetts Institute of Technology, USA.Presents results that are vital for the emerging field of valleytronics.Offers insights into the novel optical an
叢書名稱Springer Theses
圖書封面Titlebook: Coherent Light-Matter Interactions in Monolayer Transition-Metal Dichalcogenides;  Edbert Jarvis Sie Book 2018 Springer International Publi
描述This thesis presents optical methods to split the energy levels of electronic valleys in transition-metal dichalcogenides (TMDs) by means of coherent light-matter interactions. The electronic valleys found in monolayer TMDs such as MoS2, WS2, and WSe2 are among the many novel properties exhibited by semiconductors when thinned down to a few atomic layers, and have have been proposed as a new way to carry information in next generation devices (so-called valleytronics). These valleys are, however, normally locked in the same energy level, which limits their potential use for applications. The author describes experiments performed with a pump-probe technique using transient absorption spectroscopy on MoS2 and WS2. It is demonstrated that hybridizing the electronic valleys with light allows one to optically tune their energy levels in a controllable valley-selective manner. In particular, by using off-resonance circularly polarized light at small detuning, one can tune the energy level of one valley through the optical Stark effect. Also presented within are observations, at larger detuning, of a separate contribution from the so-called Bloch--Siegert effect, a delicate phenomenon th
出版日期Book 2018
關(guān)鍵詞time-resolved absorption spectroscopy; angle-resolved absorption spectroscopy; coherent light-matter i
版次1
doihttps://doi.org/10.1007/978-3-319-69554-9
isbn_softcover978-3-319-88799-9
isbn_ebook978-3-319-69554-9Series ISSN 2190-5053 Series E-ISSN 2190-5061
issn_series 2190-5053
copyrightSpringer International Publishing AG 2018
The information of publication is updating

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Intervalley Biexcitons in Monolayer MoS2, we identify two species of intervalley biexcitons with large binding energies of 60 and 40?meV. In addition, we also reveal effects beyond biexcitonic pairwise interactions in which the exciton energy redshifts at increasing exciton densities, indicating the presence of many-body interactions among
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Valley-Selective Optical Stark Effect in Monolayer WS2,pplying intense circularly polarized light, which breaks time-reversal symmetry, we demonstrate that the exciton level in each valley can be selectively tuned by as much as 18?meV via the optical Stark effect. These results offer a novel way to control valley degree of freedom and may provide a mean
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Book 2018by using off-resonance circularly polarized light at small detuning, one can tune the energy level of one valley through the optical Stark effect. Also presented within are observations, at larger detuning, of a separate contribution from the so-called Bloch--Siegert effect, a delicate phenomenon th
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Edbert Jarvis SieNominated as an outstanding Ph.D. thesis by Massachusetts Institute of Technology, USA.Presents results that are vital for the emerging field of valleytronics.Offers insights into the novel optical an
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